Attosecond spectroscopy reveals alignment dependent core-hole dynamics in the ICl molecule

Hugo J. B. Marroux; Ashley P. Fidler; Aryya Ghosh; Yuki Kobayashi; Kirill Gokhberg; Alexander I. Kuleff; Stephen R. Leone; Daniel M. Neumark

doi:10.1038/s41467-020-19496-0

Nature Communications (Nov 2020)

Attosecond spectroscopy reveals alignment dependent core-hole dynamics in the ICl molecule

Hugo J. B. Marroux,
Ashley P. Fidler,
Aryya Ghosh,
Yuki Kobayashi,
Kirill Gokhberg,
Alexander I. Kuleff,
Stephen R. Leone,
Daniel M. Neumark

Affiliations

Hugo J. B. Marroux: Department of Chemistry, University of California
Ashley P. Fidler: Department of Chemistry, University of California
Aryya Ghosh: Theoretische Chemie, PCI, Universität Heidelberg
Yuki Kobayashi: Department of Chemistry, University of California
Kirill Gokhberg: Theoretische Chemie, PCI, Universität Heidelberg
Alexander I. Kuleff: Theoretische Chemie, PCI, Universität Heidelberg
Stephen R. Leone: Department of Chemistry, University of California
Daniel M. Neumark: Department of Chemistry, University of California

DOI: https://doi.org/10.1038/s41467-020-19496-0
Journal volume & issue: Vol. 11, no. 1
pp. 1 – 8

Abstract

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Here the authors report a study measuring lifetimes of core-hole states of ICl molecule using attosecond transient absorption spectroscopy. They find that lifetimes depend on the alignment of the orbital relative to the molecular axis.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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