Nature Communications (Jan 2022)
Nano-spectroscopy of excitons in atomically thin transition metal dichalcogenides
- Shuai Zhang,
- Baichang Li,
- Xinzhong Chen,
- Francesco L. Ruta,
- Yinming Shao,
- Aaron J. Sternbach,
- A. S. McLeod,
- Zhiyuan Sun,
- Lin Xiong,
- S. L. Moore,
- Xinyi Xu,
- Wenjing Wu,
- Sara Shabani,
- Lin Zhou,
- Zhiying Wang,
- Fabian Mooshammer,
- Essance Ray,
- Nathan Wilson,
- P. J. Schuck,
- C. R. Dean,
- A. N. Pasupathy,
- Michal Lipson,
- Xiaodong Xu,
- Xiaoyang Zhu,
- A. J. Millis,
- Mengkun Liu,
- James C. Hone,
- D. N. Basov
Affiliations
- Shuai Zhang
- Department of Physics, Columbia University
- Baichang Li
- Department of Mechanical Engineering, Columbia University
- Xinzhong Chen
- National Synchrotron Light Source II, Brookhaven National Laboratory
- Francesco L. Ruta
- Department of Physics, Columbia University
- Yinming Shao
- Department of Physics, Columbia University
- Aaron J. Sternbach
- Department of Physics, Columbia University
- A. S. McLeod
- Department of Physics, Columbia University
- Zhiyuan Sun
- Department of Physics, Columbia University
- Lin Xiong
- Department of Physics, Columbia University
- S. L. Moore
- Department of Physics, Columbia University
- Xinyi Xu
- Department of Mechanical Engineering, Columbia University
- Wenjing Wu
- Department of Chemistry, Columbia University
- Sara Shabani
- Department of Physics, Columbia University
- Lin Zhou
- Department of Chemistry, Columbia University
- Zhiying Wang
- Department of Mechanical Engineering, Columbia University
- Fabian Mooshammer
- Department of Physics, Columbia University
- Essance Ray
- Department of Physics, University of Washington
- Nathan Wilson
- Department of Physics, University of Washington
- P. J. Schuck
- Department of Mechanical Engineering, Columbia University
- C. R. Dean
- Department of Physics, Columbia University
- A. N. Pasupathy
- Department of Physics, Columbia University
- Michal Lipson
- Department of Electrical Engineering, Columbia University
- Xiaodong Xu
- Department of Physics, University of Washington
- Xiaoyang Zhu
- Department of Chemistry, Columbia University
- A. J. Millis
- Department of Physics, Columbia University
- Mengkun Liu
- National Synchrotron Light Source II, Brookhaven National Laboratory
- James C. Hone
- Department of Mechanical Engineering, Columbia University
- D. N. Basov
- Department of Physics, Columbia University
- DOI
- https://doi.org/10.1038/s41467-022-28117-x
- Journal volume & issue
-
Vol. 13,
no. 1
pp. 1 – 8
Abstract
Excitons play an important role in the optical properties of 2D semiconductors, but their spatial characterization is usually constrained by the diffraction limit. Here, the authors report near-field optical spectroscopy of 2D transition metal dichalcogenides with 20 nm resolution, revealing their spatially dependent excitonic spectra and complex dielectric function.