Engineering β-ketoamine covalent organic frameworks for photocatalytic overall water splitting

Yan Yang; Xiaoyu Chu; Hong-Yu Zhang; Rui Zhang; Yu-Han Liu; Feng-Ming Zhang; Meng Lu; Zhao-Di Yang; Ya-Qian Lan

doi:10.1038/s41467-023-36338-x

Nature Communications (Feb 2023)

Engineering β-ketoamine covalent organic frameworks for photocatalytic overall water splitting

Yan Yang,
Xiaoyu Chu,
Hong-Yu Zhang,
Rui Zhang,
Yu-Han Liu,
Feng-Ming Zhang,
Meng Lu,
Zhao-Di Yang,
Ya-Qian Lan

Affiliations

Yan Yang: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Xiaoyu Chu: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Hong-Yu Zhang: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Rui Zhang: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Yu-Han Liu: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Feng-Ming Zhang: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Meng Lu: School of Chemistry, South China Normal University
Zhao-Di Yang: Heilongjiang Provincial Key Laboratory of CO2 Resource Utilization and Energy Catalytic Materials, School of Material Science and Chemical Engineering, Harbin University of Science and Technology
Ya-Qian Lan: School of Chemistry, South China Normal University

DOI: https://doi.org/10.1038/s41467-023-36338-x
Journal volume & issue: Vol. 14, no. 1
pp. 1 – 10

Abstract

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Covalent organic frameworks (COFs) are an emerging type of crystalline and porous photocatalysts for hydrogen evolution. Here, the authors report a β-ketoamine COF by systematically engineering N-sites, architecture, and morphology for improved water splitting activity.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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