Construction of a High-Performance Composite Solid Electrolyte Through In-Situ Polymerization within a Self-Supported Porous Garnet Framework

An-Giang Nguyen; Min-Ho Lee; Jaekook Kim; Chan-Jin Park

doi:10.1007/s40820-023-01294-0

Nano-Micro Letters (Jan 2024)

Construction of a High-Performance Composite Solid Electrolyte Through In-Situ Polymerization within a Self-Supported Porous Garnet Framework

An-Giang Nguyen,
Min-Ho Lee,
Jaekook Kim,
Chan-Jin Park

Affiliations

An-Giang Nguyen: Department of Materials Science and Engineering, Chonnam National University
Min-Ho Lee: Department of Materials Science and Engineering, Chonnam National University
Jaekook Kim: Department of Materials Science and Engineering, Chonnam National University
Chan-Jin Park: Department of Materials Science and Engineering, Chonnam National University

DOI: https://doi.org/10.1007/s40820-023-01294-0
Journal volume & issue: Vol. 16, no. 1
pp. 1 – 15

Abstract

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Highlights A scalable tape-casting method produces self-supported porous Li6.4La3Zr1.4Ta0.6O12. Combining the in-situ polymerization approach, a composite solid electrolyte with superior electrochemical properties is fabricated. Solid-state Li|CSE|LiNi0.8Co0.1Mn0.1O2 cells show remarkable cyclability and rate capability. LiF-and B-rich interphase layers mitigate interfacial reactions, enhancing solid-state battery performance.

Published in Nano-Micro Letters

ISSN: 2311-6706 (Print); 2150-5551 (Online)
Publisher: SpringerOpen
Country of publisher: Germany
LCC subjects: Technology
Website: http://www.springer.com/40820

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