Nature Communications (Feb 2024)

Ultracompact mirror device for forming 20-nm achromatic soft-X-ray focus toward multimodal and multicolor nanoanalyses

  • Takenori Shimamura,
  • Yoko Takeo,
  • Fumika Moriya,
  • Takashi Kimura,
  • Mari Shimura,
  • Yasunori Senba,
  • Hikaru Kishimoto,
  • Haruhiko Ohashi,
  • Kenta Shimba,
  • Yasuhiko Jimbo,
  • Hidekazu Mimura

DOI
https://doi.org/10.1038/s41467-023-44269-w
Journal volume & issue
Vol. 15, no. 1
pp. 1 – 12

Abstract

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Abstract Nanoscale soft-X-ray microscopy is a powerful analysis tool in biological, chemical, and physical sciences. To enhance its probe sensitivity and leverage multimodal soft-X-ray microscopy, precise achromatic focusing devices, which are challenging to fabricate, are essential. Here, we develop an ultracompact Kirkpatrick-Baez (ucKB) mirror, which is ideal for the high-performance nanofocusing of broadband-energy X-rays. We apply our advanced fabrication techniques and short-focal-length strategy to realize diffraction-limited focusing over the entire soft-X-ray range. We achieve a focus size of 20.4 nm at 2 keV, which represents a significant improvement in achromatic soft-X-ray focusing. The ucKB mirror extends soft-X-ray fluorescence microscopy by producing a bicolor nanoprobe with a 1- or 2-keV photon energy. We propose a subcellular chemical mapping method that allows a comprehensive analysis of specimen morphology and the distribution of light elements and metal elements. ucKB mirrors will improve soft-X-ray nanoanalyses by facilitating photon-hungry, multimodal, and polychromatic methods, even with table-top X-ray sources.