Nature Communications (May 2016)
Hetero-site-specific X-ray pump-probe spectroscopy for femtosecond intramolecular dynamics
- A. Picón,
- C. S. Lehmann,
- C. Bostedt,
- A. Rudenko,
- A. Marinelli,
- T. Osipov,
- D. Rolles,
- N. Berrah,
- C. Bomme,
- M. Bucher,
- G. Doumy,
- B. Erk,
- K. R. Ferguson,
- T. Gorkhover,
- P. J. Ho,
- E. P. Kanter,
- B. Krässig,
- J. Krzywinski,
- A. A. Lutman,
- A. M. March,
- D. Moonshiram,
- D. Ray,
- L. Young,
- S. T. Pratt,
- S. H. Southworth
Affiliations
- A. Picón
- Argonne National Laboratory
- C. S. Lehmann
- Argonne National Laboratory
- C. Bostedt
- Argonne National Laboratory
- A. Rudenko
- Department of Physics, J.R. Macdonald Laboratory, Kansas State University
- A. Marinelli
- SLAC National Accelerator Laboratory
- T. Osipov
- SLAC National Accelerator Laboratory
- D. Rolles
- Department of Physics, J.R. Macdonald Laboratory, Kansas State University
- N. Berrah
- Department of Physics, University of Connecticut
- C. Bomme
- Deutsches Elektronen-Synchrotron (DESY)
- M. Bucher
- Argonne National Laboratory
- G. Doumy
- Argonne National Laboratory
- B. Erk
- Deutsches Elektronen-Synchrotron (DESY)
- K. R. Ferguson
- SLAC National Accelerator Laboratory
- T. Gorkhover
- SLAC National Accelerator Laboratory
- P. J. Ho
- Argonne National Laboratory
- E. P. Kanter
- Argonne National Laboratory
- B. Krässig
- Argonne National Laboratory
- J. Krzywinski
- SLAC National Accelerator Laboratory
- A. A. Lutman
- SLAC National Accelerator Laboratory
- A. M. March
- Argonne National Laboratory
- D. Moonshiram
- Argonne National Laboratory
- D. Ray
- SLAC National Accelerator Laboratory
- L. Young
- Argonne National Laboratory
- S. T. Pratt
- Argonne National Laboratory
- S. H. Southworth
- Argonne National Laboratory
- DOI
- https://doi.org/10.1038/ncomms11652
- Journal volume & issue
-
Vol. 7,
no. 1
pp. 1 – 6
Abstract
Two-color X-ray pulses with controlled time delay allow exciting one site of a molecule and then probing a different site of the same molecule with femtosecond resolution. Here, the authors use this hetero-site pump-probe technique to study charge redistribution and dissociation of the xenon difluoride molecule.
