Nature Communications (Aug 2018)

Active site localization of methane oxidation on Pt nanocrystals

  • Dongjin Kim,
  • Myungwoo Chung,
  • Jerome Carnis,
  • Sungwon Kim,
  • Kyuseok Yun,
  • Jinback Kang,
  • Wonsuk Cha,
  • Mathew J. Cherukara,
  • Evan Maxey,
  • Ross Harder,
  • Kiran Sasikumar,
  • Subramanian K. R. S. Sankaranarayanan,
  • Alexey Zozulya,
  • Michael Sprung,
  • Dohhyung Riu,
  • Hyunjung Kim

DOI
https://doi.org/10.1038/s41467-018-05464-2
Journal volume & issue
Vol. 9, no. 1
pp. 1 – 7

Abstract

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The structural changes at low-coordination sites of nanocatalysts such as edges, remain poorly understood. Here, the authors report observations of high-lattice distortion at edges of Pt nanocrystals during heterogeneous catalytic methane oxidation by using in situ 3D Bragg coherent X-ray diffraction imaging.