Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols

Yinwen Li; Wa Gao; Mi Peng; Junbo Zhang; Jialve Sun; Yao Xu; Song Hong; Xi Liu; Xingwu Liu; Min Wei; Bingsen Zhang; Ding Ma

doi:10.1038/s41467-019-13691-4

Nature Communications (Jan 2020)

Interfacial Fe5C2-Cu catalysts toward low-pressure syngas conversion to long-chain alcohols

Yinwen Li,
Wa Gao,
Mi Peng,
Junbo Zhang,
Jialve Sun,
Yao Xu,
Song Hong,
Xi Liu,
Xingwu Liu,
Min Wei,
Bingsen Zhang,
Ding Ma

Affiliations

Yinwen Li: State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology
Wa Gao: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
Mi Peng: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
Junbo Zhang: State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology
Jialve Sun: State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology
Yao Xu: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
Song Hong: State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology
Xi Liu: State Key Laboratory of Coal Conversion, Institute of Coal Chemistry Chinese Academy of Sciences Taiyuan
Xingwu Liu: State Key Laboratory of Coal Conversion, Institute of Coal Chemistry Chinese Academy of Sciences Taiyuan
Min Wei: State Key Laboratory of Chemical Resource Engineering, Beijing Advanced Innovation Center for Soft Matter Science and Engineering, Beijing University of Chemical Technology
Bingsen Zhang: Shenyang National Laboratory, Institute of Metal Research, Chinese Academy of Sciences
Ding Ma: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University

DOI: https://doi.org/10.1038/s41467-019-13691-4
Journal volume & issue: Vol. 11, no. 1
pp. 1 – 8

Abstract

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Long-chain alcohols synthesis from syngas conversion is a promising route for the production of high-value chemicals. Here the authors show that a heterogeneous Fe5C2/Cu catalyst derived from layered double hydroxides precursor exhibits excellent performance with a space time yield of 0.101 g gcat −1 h−1 at a low pressure of 1 MPa.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

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