Nature Communications (Feb 2021)

Morphology and mechanism of highly selective Cu(II) oxide nanosheet catalysts for carbon dioxide electroreduction

  • Xingli Wang,
  • Katharina Klingan,
  • Malte Klingenhof,
  • Tim Möller,
  • Jorge Ferreira de Araújo,
  • Isaac Martens,
  • Alexander Bagger,
  • Shan Jiang,
  • Jan Rossmeisl,
  • Holger Dau,
  • Peter Strasser

DOI
https://doi.org/10.1038/s41467-021-20961-7
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 12

Abstract

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Copper oxides (CuO) can selectively catalyze the electrochemical reduction of CO2 to hydrocarbons and oxygenates. Here, the authors study the activity and morphological evolution of 2D CuO nanosheets under applied electrode potentials to conclude the primacy of dendritic shapes and involvement of a new coupling pathway.