Nature Communications (Feb 2017)

Decoupling absorption and emission processes in super-resolution localization of emitters in a plasmonic hotspot

  • David L. Mack,
  • Emiliano Cortés,
  • Vincenzo Giannini,
  • Peter Török,
  • Tyler Roschuk,
  • Stefan A. Maier

DOI
https://doi.org/10.1038/ncomms14513
Journal volume & issue
Vol. 8, no. 1
pp. 1 – 10

Abstract

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Reporting the position of molecules and the electromagnetic enhancement in a plasmonic hotspot is difficult. Here Macket al. use a large Stokes-shifted molecule to spectrally decouple the emission process of the dye from the plasmonic system, keeping the absorption on resonance with the plasmon resonance of the antenna.