Nature Communications (Feb 2017)
Decoupling absorption and emission processes in super-resolution localization of emitters in a plasmonic hotspot
Abstract
Reporting the position of molecules and the electromagnetic enhancement in a plasmonic hotspot is difficult. Here Macket al. use a large Stokes-shifted molecule to spectrally decouple the emission process of the dye from the plasmonic system, keeping the absorption on resonance with the plasmon resonance of the antenna.