Nanostructured gold and silver thin films were grown by pulsed laser deposition.Performing the process in an ambient gas (Ar) leads to the nucleation and growth ofnanoparticles in the ablation plasma and their self-organization on the substrate. Thedependence of surface nanostructuring of the films on the deposition parameters is discussedconsidering in particular the number of laser pulses and the ambient gas nature and pressure.The performance of the deposited thin films as substrates for surface-enhanced Ramanspectroscopy (SERS) was tested against the detection of molecules at a low concentration.Taking Raman maps on micrometer-sized areas, the spatial homogeneity of the substrateswith respect to the SERS signal was tested.
