Atmospheric Chemistry and Physics (Jun 2022)
Aerosol atmospheric rivers: climatology, event characteristics, and detection algorithm sensitivities
Abstract
Leveraging the concept of atmospheric rivers (ARs), a detection technique based on a widely utilized global algorithm to detect ARs (Guan and Waliser, 2019, 2015; Guan et al., 2018) was recently developed to detect aerosol atmospheric rivers (AARs) using the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) reanalysis (Chakraborty et al., 2021a). The current study further characterizes and quantifies various details of AARs that were not provided in that study, such as the AARs' seasonality, event characteristics, vertical profiles of aerosol mass mixing ratio and wind speed, and the fraction of total annual aerosol transport conducted by AARs. Analysis is also performed to quantify the sensitivity of AAR detection to the criteria and thresholds used by the algorithm. AARs occur more frequently over, and typically extend from, regions with higher aerosol emission. For a number of planetary-scale pathways that exhibit large climatological aerosol transport, AARs contribute up to a maximum of 80 % to the total annual transport, depending on the species of aerosols. Dust (DU) AARs are more frequent in boreal spring, sea salt AARs are often more frequent during the boreal winter (summer) in the Northern (Southern) Hemisphere, carbonaceous (CA) AARs are more frequent during dry seasons, and often originate from the global rainforests and industrial areas, and sulfate AARs are present in the Northern Hemisphere during all seasons. For most aerosol types, the mass mixing ratio within AARs is highest near the surface. However, DU and CA AARs over or near the African continent exhibit peaks in their aerosol mixing ratio profiles around 700 hPa. AAR event characteristics are mostly independent of species with the mean length, width, and length / width ratio around 4000 km, 600 km, and 7–8, respectively.