Physical Review Research (Feb 2023)

Quantum correlation of electron and ion energy in the dissociative strong-field ionization of H_{2}

  • A. Geyer,
  • O. Neufeld,
  • D. Trabert,
  • U. De Giovannini,
  • M. Hofmann,
  • N. Anders,
  • L. Sarkadi,
  • M. S. Schöffler,
  • L. Ph. H. Schmidt,
  • A. Rubio,
  • T. Jahnke,
  • M. Kunitski,
  • S. Eckart

DOI
https://doi.org/10.1103/PhysRevResearch.5.013123
Journal volume & issue
Vol. 5, no. 1
p. 013123

Abstract

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We report on the strong field ionization of H_{2} by a corotating two-color laser field. We measure the electron momentum distribution in coincidence with the kinetic energy release (KER) of dissociating hydrogen molecules. In addition to a characteristic half-moon structure, we observe a low-energy structure in the electron momentum distribution at a KER of about 3.5 eV. We speculate that the outgoing electron interacts with the molecular ion, despite the absence of classical recollisions under these conditions. Time-dependent density functional theory simulations support our conclusions.