Nature Communications (May 2018)
Ambient ammonia synthesis via palladium-catalyzed electrohydrogenation of dinitrogen at low overpotential
Abstract
The Haber-Bosch process, producing NH3 from N2, is a crucial yet energetically demanding reaction, inspiring interest in the exploration of ambient-condition alternatives. Here, authors develop a palladium electrocatalyst that shows a high selectivity and activity for N2 reduction to NH3.