Photodetector Based on CsPbBr<sub>3</sub>/Cs<sub>4</sub>PbBr<sub>6</sub> Composite Nanocrystals with High Detectivity
Yue Han,
Rong Wen,
Feng Zhang,
Linlin Shi,
Wenyan Wang,
Ting Ji,
Guohui Li,
Yuying Hao,
Lin Feng,
Yanxia Cui
Affiliations
Yue Han
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Rong Wen
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Feng Zhang
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Linlin Shi
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Wenyan Wang
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Ting Ji
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Guohui Li
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Yuying Hao
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Lin Feng
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
Yanxia Cui
College of Physics and Optoelectronics, Key Laboratory of Advanced Transducers and Intelligent Control System of Ministry of Education, Key Laboratory of Interface Science and Engineering in Advanced Materials of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, China
High-quality, all-inorganic CsPbBr3/Cs4PbBr6 composite perovskite nanocrystals (NCs) were obtained with all-solution-processing at room temperature, and a photodetector (PD) with high detectivity was realized based on CsPbBr3/Cs4PbBr6 NCs. The detectivity (D*) of the proposed PD is 4.24 × 1012 Jones under 532 nm illumination, which is among the highest levels for PDs based on all-inorganic perovskite NCs. In addition, a high linear dynamic range (LDR) of 115 dB under 1 V bias was also realized. Furthermore, the underlying mechanism for the enhanced performance of the proposed PD was discussed. Our work might promote the preparation of high-performance PDs based on dual-phase all-inorganic perovskite nanocrystals.
