Experimental observations of seed growth and accompanying pedestal contamination in a self-seeded, soft x-ray free-electron laser

Abstract

Measurements of the soft x-ray, self-seeding spectrum at the Linac Coherent Light Source (LCLS) free-electron laser generally display a pedestal-like distribution around the central seeded wavelength. This pedestal limits the spectral purity and can negatively affect some user applications not employing a post-undulator monochromator. In this paper, we investigate the detailed experimental characteristics of both the amplified seed and its accompanying pedestal using data from a number of separate LCLS shifts over the 2015-2018 time period. We find that the amplified seed shows excellent wavelength stability and an exponential growth rate whose dependence upon energy detuning is consistent with theory. The pedestal’s spectral distribution and integrated strength vary strongly shot by shot, independent of electron beam energy jitter. Its shot-averaged strength relative to that of the seed grows at least linearly with z and can approach values of 15% or more. The pedestal is comprised of two separate components: (1) normal self-amplified spontaneous emission (SASE) whose total strength is nominally insensitive to energy detuning and laser heater (LH) strength; (2) sideband-like emission whose strength positively correlates with that of the amplified seed and negatively with energy detuning and LH strength. We believe this latter, non-SASE component arises from comparatively long wavelength (i.e., λ∼0.3–3 μm) amplitude and phase modulations of the main seeded radiation line. Its shot to shot variability and LH sensitivity suggests an origin connected to growth of the longitudinal microbunching instability on the electron beam.