Carbon Resources Conversion (Jun 2024)

Controlled fabrication of Fe3N@NG composites as superior oxygen evolution reaction electrocatalysts

  • Yang Song,
  • Tongya Tian,
  • Changming Li,
  • Xi Zeng,
  • Sen Zhang,
  • Li Chen,
  • Zhenghua Yang,
  • Qizhe Ji,
  • Xianglong Zhao,
  • Feiyong Chen

Journal volume & issue
Vol. 7, no. 2
p. 100207

Abstract

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We report the controlled fabrication of nitrogen doped graphene (NG) nanoplates, which are uniformly decorated with iron nitride (Fe3N) nanoparticles, via ball milling of mixtures of graphite and iron nitrates and the following ammonia annealing. The obtained Fe3N@NG composites demonstrate excellent electrocatalytic activity and durability for oxygen evolution reaction, both of which outperform those of the state-of-the-art iridium oxide catalysts. This may be attributed to nitrogen doping as well as the synergistic effect between Fe3N and graphene nanoplates.

Keywords