Near 100% ethene selectivity achieved by tailoring dual active sites to isolate dehydrogenation and oxidation

Chaojie Wang; Bing Yang; Qingqing Gu; Yujia Han; Ming Tian; Yang Su; Xiaoli Pan; Yu Kang; Chuande Huang; Hua Liu; Xiaoyan Liu; Lin Li; Xiaodong Wang

doi:10.1038/s41467-021-25782-2

Nature Communications (Sep 2021)

Near 100% ethene selectivity achieved by tailoring dual active sites to isolate dehydrogenation and oxidation

Chaojie Wang,
Bing Yang,
Qingqing Gu,
Yujia Han,
Ming Tian,
Yang Su,
Xiaoli Pan,
Yu Kang,
Chuande Huang,
Hua Liu,
Xiaoyan Liu,
Lin Li,
Xiaodong Wang

Affiliations

Chaojie Wang: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Bing Yang: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Qingqing Gu: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Yujia Han: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Ming Tian: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Yang Su: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Xiaoli Pan: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Yu Kang: Max Planck Institute for Chemical Physics of Solids
Chuande Huang: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Hua Liu: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Xiaoyan Liu: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Lin Li: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
Xiaodong Wang: CAS Key Laboratory of Science and Technology on Applied Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences

DOI: https://doi.org/10.1038/s41467-021-25782-2
Journal volume & issue: Vol. 12, no. 1
pp. 1 – 8

Abstract

Read online

It is important but challenging to prohibit deep oxidation of alkene in oxidative dehydrogenation of light alkane. Here, dual active sites are tailored to isolate dehydrogenation and oxidation thus achieving superior ethene selectivity.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

About the journal