Nature Communications (Dec 2016)

A metal-free electrocatalyst for carbon dioxide reduction to multi-carbon hydrocarbons and oxygenates

  • Jingjie Wu,
  • Sichao Ma,
  • Jing Sun,
  • Jake I. Gold,
  • ChandraSekhar Tiwary,
  • Byoungsu Kim,
  • Lingyang Zhu,
  • Nitin Chopra,
  • Ihab N. Odeh,
  • Robert Vajtai,
  • Aaron Z. Yu,
  • Raymond Luo,
  • Jun Lou,
  • Guqiao Ding,
  • Paul J. A. Kenis,
  • Pulickel M. Ajayan

DOI
https://doi.org/10.1038/ncomms13869
Journal volume & issue
Vol. 7, no. 1
pp. 1 – 6

Abstract

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Electroreduction of CO2 into C2 hydrocarbons and liquid fuels is a promising but challenging energy conversion technology, with copper exhibiting fair selectivity for these products. Here, the authors report that N-doped graphene quantum dots can also catalyze the electrochemical reduction of CO2into multi-carbon hydrocarbons and oxygenates.