Effect of Applied DC Electric Fields on H₂–Air Axisymmetric Laminar Co-Flow Diffusion Flames with Low Carbon Impurities

Abstract

We investigated experimentally the influence of flow conditions and electrode position on a diffusion H2–air flame subjected to an external electric field. We determined the minimum impurity level required to observe changes in flame properties with applied voltage. Flame OH chemiluminescence signals were recorded using a UV-sensitive CCD array as a function of voltage (+10 to −10 kV) applied to a stainless-steel ring electrode placed around the burner nozzle. Changes in chemiluminescence signals are reported as a function of electrode height above the burner, airflow, and fuel composition. Significant changes in OH* distributions were observed for voltages below −5 kV. Under optimum conditions, the height of the chemiluminescence flame decreased by up to 67% at the maximum applied voltage. The flame transitioned from a teardrop shape to a flat, open-tip flame at a voltage corresponding to an inflection point in the flame height–voltage profiles. Increasing the airflow rate shifted the inflection point to more negative values until almost suppressing the effect of the electric field on the flame structure. This study reveals that carbon impurities in hydrogen fuel as low as 10 ppm are sufficient to observe significant effects from external electric fields without changing the underlying neutral chemistry. We also determine the set of parameters that control the amplitude of the structural change.

Keywords

• electric field
• hydrogen flame
• co-flow burner
• diffusion flame
• chemiluminescence