Nature Communications (Aug 2021)
Stabilizing the framework of SAPO-34 zeolite toward long-term methanol-to-olefins conversion
- Liu Yang,
- Chang Wang,
- Lina Zhang,
- Weili Dai,
- Yueying Chu,
- Jun Xu,
- Guangjun Wu,
- Mingbin Gao,
- Wenjuan Liu,
- Zhaochao Xu,
- Pengfei Wang,
- Naijia Guan,
- Michael Dyballa,
- Mao Ye,
- Feng Deng,
- Weibin Fan,
- Landong Li
Affiliations
- Liu Yang
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Chang Wang
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Lina Zhang
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Weili Dai
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Yueying Chu
- National Center for Magnetic Resonance in Wuhan, State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Key Laboratory of Magnetic Resonance in Biological Systems, Wuhan Institute of Physics and Mathematics, Chinese Academy of Sciences
- Jun Xu
- National Center for Magnetic Resonance in Wuhan, State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Key Laboratory of Magnetic Resonance in Biological Systems, Wuhan Institute of Physics and Mathematics, Chinese Academy of Sciences
- Guangjun Wu
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Mingbin Gao
- Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Wenjuan Liu
- Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Zhaochao Xu
- Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Pengfei Wang
- State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences
- Naijia Guan
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- Michael Dyballa
- Institute of Chemical Technology, University of Stuttgart
- Mao Ye
- Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Feng Deng
- National Center for Magnetic Resonance in Wuhan, State Key Laboratory of Magnetic Resonance and Atomic and Molecular Physics, Key Laboratory of Magnetic Resonance in Biological Systems, Wuhan Institute of Physics and Mathematics, Chinese Academy of Sciences
- Weibin Fan
- State Key Laboratory of Coal Conversion, Institute of Coal Chemistry, Chinese Academy of Sciences
- Landong Li
- School of Materials Science and Engineering, and National Institute for Advanced Materials, Nankai University
- DOI
- https://doi.org/10.1038/s41467-021-24403-2
- Journal volume & issue
-
Vol. 12,
no. 1
pp. 1 – 11
Abstract
Stability of zeolite catalysts is a highly desirable property for commercial methanol to olefins conversion but extremely challenging to achieve. Here, the authors combine the catalyst pre-coking and water co-feeding to develop an efficient strategy to enhance the long-term stability of SAPO-34 catalyst.