Nature Communications (Jan 2023)
Selective CO2 electrolysis to CO using isolated antimony alloyed copper
- Jiawei Li,
- Hongliang Zeng,
- Xue Dong,
- Yimin Ding,
- Sunpei Hu,
- Runhao Zhang,
- Yizhou Dai,
- Peixin Cui,
- Zhou Xiao,
- Donghao Zhao,
- Liujiang Zhou,
- Tingting Zheng,
- Jianping Xiao,
- Jie Zeng,
- Chuan Xia
Affiliations
- Jiawei Li
- School of Materials and Energy, University of Electronic Science and Technology of China
- Hongliang Zeng
- School of Materials and Energy, University of Electronic Science and Technology of China
- Xue Dong
- State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, University of Chinese Academy of Sciences, Dalian National Laboratory for Clean Energy
- Yimin Ding
- Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China
- Sunpei Hu
- Hefei National Research Center for Physical Sciences at the Microscale, Key Laboratory of Strongly Coupled Quantum Matter Physics of Chinese Academy of Sciences, National Synchrotron Radiation Laboratory, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Runhao Zhang
- School of Materials and Energy, University of Electronic Science and Technology of China
- Yizhou Dai
- School of Materials and Energy, University of Electronic Science and Technology of China
- Peixin Cui
- Key Laboratory of Soil Environment and Pollution Remediation, Institute of Soil Science, Chinese Academy of Sciences
- Zhou Xiao
- Hefei National Research Center for Physical Sciences at the Microscale, Key Laboratory of Strongly Coupled Quantum Matter Physics of Chinese Academy of Sciences, National Synchrotron Radiation Laboratory, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Donghao Zhao
- Hefei National Research Center for Physical Sciences at the Microscale, Key Laboratory of Strongly Coupled Quantum Matter Physics of Chinese Academy of Sciences, National Synchrotron Radiation Laboratory, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Liujiang Zhou
- Yangtze Delta Region Institute (Huzhou), University of Electronic Science and Technology of China
- Tingting Zheng
- School of Materials and Energy, University of Electronic Science and Technology of China
- Jianping Xiao
- State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, University of Chinese Academy of Sciences, Dalian National Laboratory for Clean Energy
- Jie Zeng
- Hefei National Research Center for Physical Sciences at the Microscale, Key Laboratory of Strongly Coupled Quantum Matter Physics of Chinese Academy of Sciences, National Synchrotron Radiation Laboratory, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Chuan Xia
- School of Materials and Energy, University of Electronic Science and Technology of China
- DOI
- https://doi.org/10.1038/s41467-023-35960-z
- Journal volume & issue
-
Vol. 14,
no. 1
pp. 1 – 11
Abstract
Engineering Cu to achieve high catalytic selectivity towards carbon monoxide at high current density is challenging. Here, the authors report an Cu-Sb single-atom alloy catalyst that catalyzes CO2 reduction at a current density of 500 mA cm−2 with CO FE of ca. 91%.