The Contents of Potentially Toxic Elements and Emission Characteristics of PM_2.5 in Soil Fugitive Dust around Six Cities of the Yunnan-Guizhou Plateau in China

Abstract

The contents of potentially toxic elements (V, Cr, Mn, Co, Ni, Cu, Zn, As, Cd, and Pb) and emission characteristics of PM2.5 in soil fugitive dust (SFD) in six Yunnan cities (Baoshan, Kunming, Wenshan, Honghe, Yuxi, and Zhaotong) were investigated in this research. The results showed that the contents of Zn and Pb in PM2.5 of SFD were the highest around Honghe and Yuxi, respectively, while the contents of Mn were the highest in PM2.5 of SFD around the other four cities. The enrichment factor and correlation indicated that the potentially toxic elements’ pollution degrees of PM2.5 of SFD around Kunming, Yuxi, and Honghe were higher than those around the other three cities and that potentially toxic elements were generally affected by metal smelting activities, and in Zhaotong, were affected by coal burning activities, while in Wenshan and Baoshan were less affected by human activities. The total emission of PM2.5 of SFD in the six cities was 7705.49 t in 2018. The total emission factor of PM2.5 of SFD reached the highest level from January to May and the lowest level from July to October. The health risk assessment showed that the potentially toxic elements in PM2.5 of SFD for children in the six cities and for adults in Baoshan, Kunming, Honghe, and Zhaotong had non-carcinogenic risk (non-carcinogenic risk thresholds were greater than 1), and As contributes most to non-carcinogenic risk. The carcinogenic risk value of Cr in PM2.5 of SFD in Kunming and Zhaotong was between 1 × 10−6 and 1 × 10−4, which had a certain carcinogenic risk. More attention should be paid to alleviate health risks posed by particle-bound potentially toxic elements through SFD.

Keywords

• Yunnan-Guizhou plateau
• soil fugitive dust
• PM_2.5
• potentially toxic elements
• emission characteristics
• health risk assessment