Crystals (Dec 2022)

Pressure-Induced Superconductivity in PdTeI with Quasi-One-Dimensional PdTe Chains

  • Yi Zhao,
  • Jun Hou,
  • Yang Fu,
  • Cuiying Pei,
  • Jianping Sun,
  • Qi Wang,
  • Lingling Gao,
  • Weizheng Cao,
  • Changhua Li,
  • Shihao Zhu,
  • Mingxin Zhang,
  • Yulin Chen,
  • Hechang Lei,
  • Jinguang Cheng,
  • Yanpeng Qi

DOI
https://doi.org/10.3390/cryst12121833
Journal volume & issue
Vol. 12, no. 12
p. 1833

Abstract

Read online

The quasi-one-dimensional material PdTeI exhibits unusual electronic transport properties at ambient pressure. Here, we systematically investigate both the structural and electronic responses of PdTeI to external pressure, through a combination of electrical transport, synchrotron X-ray diffraction (XRD), and Raman spectroscopy measurements. The charge density wave (CDW) order in PdTeI is fragile and the transition temperature TCDW decreases rapidly with the application of external pressure. The resistivity hump is indiscernible when the pressure is increased to ~1 GPa. Upon further compression, the resistivity dropping is observed approximately ~15 GPa and zero resistance is established above ~20 GPa, suggesting the occurrence of superconductivity. Combined XRD and Raman data evidence that the emergence of superconductivity is accompanied by a pressure-induced amorphization of PdTeI.

Keywords