Nanomaterials (Jan 2022)

Anisotropic Radiation in Heterostructured “Emitter in a Cavity” Nanowire

  • Alexey Kuznetsov,
  • Prithu Roy,
  • Valeriy M. Kondratev,
  • Vladimir V. Fedorov,
  • Konstantin P. Kotlyar,
  • Rodion R. Reznik,
  • Alexander A. Vorobyev,
  • Ivan S. Mukhin,
  • George E. Cirlin,
  • Alexey D. Bolshakov

DOI
https://doi.org/10.3390/nano12020241
Journal volume & issue
Vol. 12, no. 2
p. 241

Abstract

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Tailorable synthesis of axially heterostructured epitaxial nanowires (NWs) with a proper choice of materials allows for the fabrication of novel photonic devices, such as a nanoemitter in the resonant cavity. An example of the structure is a GaP nanowire with ternary GaPAs insertions in the form of nano-sized discs studied in this work. With the use of the micro-photoluminescence technique and numerical calculations, we experimentally and theoretically study photoluminescence emission in individual heterostructured NWs. Due to the high refractive index and near-zero absorption through the emission band, the photoluminescence signal tends to couple into the nanowire cavity acting as a Fabry–Perot resonator, while weak radiation propagating perpendicular to the nanowire axis is registered in the vicinity of each nano-sized disc. Thus, within the heterostructured nanowire, both amplitude and spectrally anisotropic photoluminescent signals can be achieved. Numerical modeling of the nanowire with insertions emitting in infrared demonstrates a decay in the emission directivity and simultaneous rise of the emitters coupling with an increase in the wavelength. The emergence of modulated and non-modulated radiation is discussed, and possible nanophotonic applications are considered.

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