Nature Communications (May 2022)
Atomic overlayer of permeable microporous cuprous oxide on palladium promotes hydrogenation catalysis
- Kunlong Liu,
- Lizhi Jiang,
- Wugen Huang,
- Guozhen Zhu,
- Yue-Jiao Zhang,
- Chaofa Xu,
- Ruixuan Qin,
- Pengxin Liu,
- Chengyi Hu,
- Jingjuan Wang,
- Jian-Feng Li,
- Fan Yang,
- Gang Fu,
- Nanfeng Zheng
Affiliations
- Kunlong Liu
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Lizhi Jiang
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Wugen Huang
- State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Guozhen Zhu
- Department of Mechanical Engineering and Manitoba Institute of Materials, University of Manitoba
- Yue-Jiao Zhang
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Chaofa Xu
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Ruixuan Qin
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Pengxin Liu
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Chengyi Hu
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Jingjuan Wang
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Jian-Feng Li
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Fan Yang
- State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences
- Gang Fu
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- Nanfeng Zheng
- State Key Laboratory for Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and National & Local Joint Engineering Research Center for Preparation Technology of Nanomaterials, College of Chemistry and Chemical Engineering, Xiamen University
- DOI
- https://doi.org/10.1038/s41467-022-30327-2
- Journal volume & issue
-
Vol. 13,
no. 1
pp. 1 – 8
Abstract
It remains a challenge to fabricate metal catalysts with interfacial active sites distributed on the whole two-dimensional (2D) surface of metal nanoparticles. Here the authors demonstrate that the overgrowth of atomic-thick porous Cu2O on Pd readily creates an unprecedented 2D catalytically active metal-support interface with significantly enhanced catalysis toward the semi-hydrogenation of alkynes.
