Nature Communications (Mar 2023)
Sustainable methane utilization technology via photocatalytic halogenation with alkali halides
- Jun Ma,
- Can Zhu,
- Keke Mao,
- Wenbin Jiang,
- Jingxiang Low,
- Delong Duan,
- Huanxin Ju,
- Dong Liu,
- Kun Wang,
- Yijing Zang,
- Shuangming Chen,
- Hui Zhang,
- Zeming Qi,
- Ran Long,
- Zhi Liu,
- Li Song,
- Yujie Xiong
Affiliations
- Jun Ma
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Can Zhu
- Department of Chemistry, Fudan University
- Keke Mao
- School of Energy and Environment Science, Anhui University of Technology
- Wenbin Jiang
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Jingxiang Low
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Delong Duan
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Huanxin Ju
- PHI China Analytical Laboratory, CoreTech Integrated Limited
- Dong Liu
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Kun Wang
- Department of Chemistry, Fudan University
- Yijing Zang
- School of Physical Science and Technology, ShanghaiTech University
- Shuangming Chen
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Hui Zhang
- State Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences
- Zeming Qi
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Ran Long
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Zhi Liu
- School of Physical Science and Technology, ShanghaiTech University
- Li Song
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- Yujie Xiong
- School of Chemistry and Materials Science, National Synchrotron Radiation Laboratory, School of Nuclear Science and Technology, University of Science and Technology of China
- DOI
- https://doi.org/10.1038/s41467-023-36977-0
- Journal volume & issue
-
Vol. 14,
no. 1
pp. 1 – 8
Abstract
A sustainable photocatalytic methane halogenation strategy is developed for methyl halide production using low-cost alkali halides over Cu-doped TiO2 nanostructures. Copper sites ultimately stabilize *CH3 to promote reaction with Cl− to form CH3Cl.
