Nature Communications (Jan 2023)
Stabilizing copper sites in coordination polymers toward efficient electrochemical C-C coupling
- Yongxiang Liang,
- Jiankang Zhao,
- Yu Yang,
- Sung-Fu Hung,
- Jun Li,
- Shuzhen Zhang,
- Yong Zhao,
- An Zhang,
- Cheng Wang,
- Dominique Appadoo,
- Lei Zhang,
- Zhigang Geng,
- Fengwang Li,
- Jie Zeng
Affiliations
- Yongxiang Liang
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Jiankang Zhao
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Yu Yang
- School of Chemical and Biomolecular Engineering and The University of Sydney Nano Institute, The University of Sydney
- Sung-Fu Hung
- Department of Applied Chemistry, National Yang Ming Chiao Tung University
- Jun Li
- Frontiers Science Center for Transformative Molecules, Shanghai Jiao Tong University
- Shuzhen Zhang
- School of Chemical and Biomolecular Engineering and The University of Sydney Nano Institute, The University of Sydney
- Yong Zhao
- School of Chemical and Biomolecular Engineering and The University of Sydney Nano Institute, The University of Sydney
- An Zhang
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Cheng Wang
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Dominique Appadoo
- Australian Synchrotron
- Lei Zhang
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Zhigang Geng
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- Fengwang Li
- School of Chemical and Biomolecular Engineering and The University of Sydney Nano Institute, The University of Sydney
- Jie Zeng
- Hefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Strongly-Coupled Quantum Matter Physics, Key Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education Institutes, Department of Chemical Physics, University of Science and Technology of China
- DOI
- https://doi.org/10.1038/s41467-023-35993-4
- Journal volume & issue
-
Vol. 14,
no. 1
pp. 1 – 10
Abstract
Typically, Cu catalysts agglomerate under electrochemical conditions. Here, the authors report a coordination polymer catalyst with neighboring Cu sites which remain isolated and reduce CO2 to C2H4 with high selectivity and stability