Dispersive coherent Brillouin scattering spectroscopy

Abstract

Frequency- and time-domain Brillouin scattering spectroscopy are powerful tools to read out the mechanical properties of complex systems in material and life sciences. Indeed, coherent acoustic phonons in the time-domain method offer superior depth resolution and a stronger signal than incoherent acoustic phonons in the frequency-domain method. However, it requires scanning of delay time between laser pulses for pumping and probing coherent acoustic phonons. Here, we present Brillouin scattering spectroscopy that spans the time and frequency domains to allow the multichannel detection of Brillouin scattering light from coherent acoustic phonons. Our technique traces the time-evolve Brillouin oscillations at the instantaneous frequency of a chromatic-dispersed laser pulse. The spectroscopic heterodyning of Brillouin scattering light in the frequency domain allows a single-frame readout of gigahertz-frequency oscillations with a spectrometer. As a proof of concept, we imaged heterogeneous thin films and biological cells over a wide bandwidth with nanometer depth resolution.

Keywords

• Brillouin microscopy
• Brillouin light scattering
• Brillouin oscillations
• Picosecond ultrasonics
• Phonon spectroscopy
• Chirped pulse spectroscopy