Strategies for improving photocatalytic performance of g-C3N4 by modulating charge separation and current research status
Shuangying Chen,
Xuliang Zhang,
Degang Li,
Xiaowen Wang,
Bingjie Hu,
Fushui Guo,
Liantao Hao,
Bo Liu
Affiliations
Shuangying Chen
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Xuliang Zhang
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China; Laboratory of Functional Molecules and Materials, School of Physics and Optoelectronic Engineering, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China; Corresponding author. Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China.
Degang Li
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Xiaowen Wang
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Bingjie Hu
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Fushui Guo
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Liantao Hao
Analysis and Testing Center, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China
Bo Liu
Laboratory of Functional Molecules and Materials, School of Physics and Optoelectronic Engineering, Shandong University of Technology, 266 Xincun Xi road, Zibo, 255000, PR China; Corresponding author.
Graphitic carbon nitride (g-C3N4) has been extensively investigated over the past decade for its potential utilizations in photocatalytic energy generation and pollutant degradation. To better meeting the requirements for practical utilizations, it is crucial to address the issue of poor charge separation properties in g-C3N4, which origin from the strong interactions in photogenerated electron-hole pairs. In this review, we summarized the pertinent studies on developing strategies to promote the charge separation properties of g-C3N4. The strategies can be categorized into two categories of promoting the surface migration of charge carriers and prolonging the lifetime of surface charge. Finally, we present potential challenges in promoting charge separation and offer feasible suggestions to face these challenges.