Nature Communications (Apr 2021)

On the limitations in assessing stability of oxygen evolution catalysts using aqueous model electrochemical cells

  • Julius Knöppel,
  • Maximilian Möckl,
  • Daniel Escalera-López,
  • Kevin Stojanovski,
  • Markus Bierling,
  • Thomas Böhm,
  • Simon Thiele,
  • Matthias Rzepka,
  • Serhiy Cherevko

DOI
https://doi.org/10.1038/s41467-021-22296-9
Journal volume & issue
Vol. 12, no. 1
pp. 1 – 9

Abstract

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Dissolution of Ir catalysts varies widely between PEM water electrolysers and aqueous electrolytes. Here, we systematically investigate this finding and propose that stabilization of the catalysts over time and overestimated ionomer acidity are the main contributors to the dissolution discrepancy.