Environmental Research Letters (Jan 2024)

Observed decade-long improvement of combustion efficiency in the Yangtze River Delta region in China

  • Jiarui Zhao,
  • Huilin Chen,
  • Ximeng Qi,
  • Xuguang Chi,
  • Mengwei Jia,
  • Fei Jiang,
  • Sheng Zhong,
  • Bo Zheng,
  • Aijun Ding

DOI
https://doi.org/10.1088/1748-9326/ad521e
Journal volume & issue
Vol. 19, no. 7
p. 074001

Abstract

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The ΔCO/ΔCO _2 ratio is a good indicator of the combustion efficiency of carbon-containing fuels, and can be useful to assess the combustion efficiency on a regional scale. In this study, we analyzed in-situ observations of CO _2 and CO concentrations from 2011 to 2021 at the Station for Observing Regional Processes of the Earth System (SORPES), in the Yangtze River Delta (YRD) region of eastern China, and calculated the ΔCO/ΔCO _2 ratio to investigate the combustion efficiency in the YRD region. Furthermore, we used a Lagrangian particle dispersion model WRF-FLEXPART to evaluate the contribution of each emission sources to the observed ΔCO/ΔCO _2 ratio. We found that the observed ΔCO/ΔCO _2 ratio showed a persistent decreasing trend of 1.0 ppb/ppm per year and decreased ∼47.9% during this period, illustrating an evident improvement in the combustion efficiency in the YRD region. The improvement of the combustion efficiency is a result of China’s Air Pollution Prevention and Control Action Plan announced in 2013. However, the decrease of ΔCO/ΔCO _2 ratio slowed down from 1.3 ppb ppm ^−1 per year during 2011–2016 to 0.6 ppb ppm ^−1 per year during 2017–2021. The simulation results reveal that the slowdown of the decrease in the ΔCO/ΔCO _2 ratios can be explained by the slowing improvement of combustion efficiency in steel source in the industry sector. Our results verify the effectiveness of emission reduction efforts in the YRD region and highlight the necessity of long-term observations of CO _2 and CO.

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