Catalysts (Jan 2023)

Recent Advances in g-C<sub>3</sub>N<sub>4</sub>-Based Photocatalysts for NO<sub>x</sub> Removal

  • Zhanyong Gu,
  • Mengdie Jin,
  • Xin Wang,
  • Ruotong Zhi,
  • Zhenghao Hou,
  • Jing Yang,
  • Hongfang Hao,
  • Shaoyan Zhang,
  • Xionglei Wang,
  • Erpeng Zhou,
  • Shu Yin

DOI
https://doi.org/10.3390/catal13010192
Journal volume & issue
Vol. 13, no. 1
p. 192

Abstract

Read online

Nitrogen oxides (NOx) pollutants can cause a series of environmental issues, such as acid rain, ground-level ozone pollution, photochemical smog and global warming. Photocatalysis is supposed to be a promising technology to solve NOx pollution. Graphitic carbon nitride (g-C3N4) as a metal-free photocatalyst has attracted much attention since 2009. However, the pristine g-C3N4 suffers from poor response to visible light, rapid charge carrier recombination, small specific surface areas and few active sites, which results in deficient solar light efficiency and unsatisfactory photocatalytic performance. In this review, we summarize and highlight the recent advances in g-C3N4-based photocatalysts for photocatalytic NOx removal. Firstly, we attempt to elucidate the mechanism of the photocatalytic NOx removal process and introduce the metal-free g-C3N4 photocatalyst. Then, different kinds of modification strategies to enhance the photocatalytic NOx removal performance of g-C3N4-based photocatalysts are summarized and discussed in detail. Finally, we propose the significant challenges and future research topics on g-C3N4-based photocatalysts for photocatalytic NOx removal, which should be further investigated and resolved in this interesting research field.

Keywords