Nature Communications (Jun 2022)

Subsurface oxygen defects electronically interacting with active sites on In2O3 for enhanced photothermocatalytic CO2 reduction

  • Weiqin Wei,
  • Zhen Wei,
  • Ruizhe Li,
  • Zhenhua Li,
  • Run Shi,
  • Shuxin Ouyang,
  • Yuhang Qi,
  • David Lee Philips,
  • Hong Yuan

DOI
https://doi.org/10.1038/s41467-022-30958-5
Journal volume & issue
Vol. 13, no. 1
pp. 1 – 12

Abstract

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How to effectively extract electrons from subsurface oxygen defects is challenging in heterogeneous catalysis. Here the authors demonstrate that Metallic In-embedded In2O3 nanoflake catalyst promotes the delocalization of electrons among subsurface oxygen defects, obviously increasing electron density of surface active sites.