EPJ Web of Conferences (Jan 2020)

Determining spontaneous fission properties by direct mass measurements with the FRS Ion Catcher

  • Mardor Israel,
  • Dickel Timo,
  • Amanbayev Daler,
  • Ayet San Andrés Samuel,
  • Beck Sönke,
  • Benyamin David,
  • Bergmann Julian,
  • Constantin Paul,
  • Cléroux Cuillerier Alexandre,
  • Geissel Hans,
  • Gröff Lizzy,
  • Hornung Christine,
  • Kripko-Koncz Gabriella,
  • Mollaebrahimi Ali,
  • Miskun Ivan,
  • Plaß Wolfgang R.,
  • Pomp Stephan,
  • Rotaru Adrian,
  • Scheidenberger Christoph,
  • Stanic Goran,
  • Will Christian

DOI
https://doi.org/10.1051/epjconf/202023902004
Journal volume & issue
Vol. 239
p. 02004

Abstract

Read online

We present a direct method to measure fission product yield distributions (FPY) and isomeric yield ratios (IYR) for spontaneous fission (SF) fragments. These physical properties are of utmost importance to the understanding of basic nuclear physics, the astrophysical rapid neutron capture process ('r process') of nucleosynthesis, neutron star composition, and nuclear reactor safety. With this method, fission fragments are produced by spontaneous fission from a source that is mounted in a cryogenic stopping cell (CSC), thermalized and stopped within it, and then extracted and transported to a multiple-reflection time-of-flight mass-spectrometer (MR-TOF-MS). We will implement the method at the FRS Ion Catcher (FRS-IC) at GSI (Germany), whose MR-TOF-MS relative mass accuracy (~ 10-7) and resolving power (~ 600,000 FWHM) are sufficient to separate all isobars and numerous isomers in the fission fragment realm. The system's essential element independence and its fast simultaneous mass measurement provide a new direct way to measure isotopic FPY distributions, which is complementary to existing methods. It will enable nuclide FPY measurements in the high fission peak, which is hardly accessible by current techniques. The extraction time of the CSC, tens of milliseconds, enables a direct measurement of independent fission yields, and a first study of the temporal dependence of FPY distributions in this duration range. The ability to resolve isomers will further enable direct extraction of numerous IYRs while performing the FPY measurements. The method has been recently demonstrated at the FRS-ICr for SF with a 37 kBq 252Cf fission source, where about 70 different fission fragments have been identified and counted. In the near future, it will be used for systematic studies of SF with a higher-activity 252Cf source and a 248Cm source. The method can be implemented also for neutron induced fission at appropriate facilities.