Green Energy & Environment (Dec 2023)

Temperature-regulation liquid gating membrane with controllable gas/liquid separation

  • Baiyi Chen,
  • Huimeng Wang,
  • Jiadai Xu,
  • Liting Pan,
  • Yuan Jing,
  • Xu Hou

Journal volume & issue
Vol. 8, no. 6
pp. 1501 – 1508

Abstract

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Membrane separation technology with the ability to regulate gas/liquid transport and separation is critical for environmental fields, such as sewerage treatment, multiphase separation, and desalination. Although numerous membranes can dynamically control liquid-phase fluids transport via external stimuli, the transport and separation of gas-phase fluids remains a challenge. Here, we show a temperature-regulation liquid gating membrane that allows in-situ dynamically controllable gas/liquid transfer and multiphase separation by integrating a thermo-wettability responsive porous membrane with functional gating liquid. Experiments and theoretical analysis have demonstrated the temperature-regulation mechanism of this liquid gating system, which is based on thermo-responsive changes of porous membrane surface polarity, leading to changes in affinity between the porous membrane and the gating liquid. In addition, the sandwich configuration with dense Au-coated surfaces and heterogeneous internal components by a bistable interface design enables the liquid gating system to enhance response sensitivity and maintain working stability. This temperature-regulation gas/liquid transfer strategy expands the application range of liquid gating membranes, which are promising in environmental governance, water treatment and multiphase separation.

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