Frontiers in Chemistry (Aug 2022)
On the adsorption and reactivity of element 114, flerovium
- A. Yakushev,
- A. Yakushev,
- L. Lens,
- L. Lens,
- Ch. E. Düllmann,
- Ch. E. Düllmann,
- Ch. E. Düllmann,
- J. Khuyagbaatar,
- J. Khuyagbaatar,
- E. Jäger,
- J. Krier,
- J. Runke,
- J. Runke,
- H. M. Albers,
- M. Asai,
- M. Block,
- M. Block,
- M. Block,
- J. Despotopulos,
- A. Di Nitto,
- A. Di Nitto,
- K. Eberhardt,
- U. Forsberg,
- P. Golubev,
- M. Götz,
- M. Götz,
- M. Götz,
- S. Götz,
- S. Götz,
- S. Götz,
- H. Haba,
- L. Harkness-Brennan,
- R.-D. Herzberg,
- F. P. Heßberger,
- F. P. Heßberger,
- D. Hinde,
- A. Hübner,
- D. Judson,
- B. Kindler,
- Y. Komori,
- J. Konki,
- J.V. Kratz,
- N. Kurz,
- M. Laatiaoui,
- M. Laatiaoui,
- M. Laatiaoui,
- S. Lahiri,
- B. Lommel,
- M. Maiti,
- A. K. Mistry,
- A. K. Mistry,
- Ch. Mokry,
- Ch. Mokry,
- K. J. Moody,
- Y. Nagame,
- J. P. Omtvedt,
- P. Papadakis,
- V. Pershina,
- D. Rudolph,
- L.G. Samiento,
- T.K. Sato,
- M. Schädel,
- P. Scharrer,
- P. Scharrer,
- P. Scharrer,
- B. Schausten,
- D. A. Shaughnessy,
- J. Steiner,
- P. Thörle-Pospiech,
- P. Thörle-Pospiech,
- A. Toyoshima,
- N. Trautmann,
- K. Tsukada,
- J. Uusitalo,
- K.-O. Voss,
- A. Ward,
- M. Wegrzecki,
- N. Wiehl,
- N. Wiehl,
- E. Williams,
- V. Yakusheva,
- V. Yakusheva
Affiliations
- A. Yakushev
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- A. Yakushev
- Helmholtz-Institut Mainz, Mainz, Germany
- L. Lens
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- L. Lens
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- Ch. E. Düllmann
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- Ch. E. Düllmann
- Helmholtz-Institut Mainz, Mainz, Germany
- Ch. E. Düllmann
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- J. Khuyagbaatar
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- J. Khuyagbaatar
- Helmholtz-Institut Mainz, Mainz, Germany
- E. Jäger
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- J. Krier
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- J. Runke
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- J. Runke
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- H. M. Albers
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Asai
- Japan Atomic Energy Agency, Tokai, Japan
- M. Block
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Block
- Helmholtz-Institut Mainz, Mainz, Germany
- M. Block
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- J. Despotopulos
- Lawrence Livermore National Laboratory, Livermore, CA, United States
- A. Di Nitto
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- A. Di Nitto
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- K. Eberhardt
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- U. Forsberg
- Lund University, Lund, Sweden
- P. Golubev
- Lund University, Lund, Sweden
- M. Götz
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Götz
- Helmholtz-Institut Mainz, Mainz, Germany
- M. Götz
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- S. Götz
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- S. Götz
- Helmholtz-Institut Mainz, Mainz, Germany
- S. Götz
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- H. Haba
- RIKEN, Wako, Japan
- L. Harkness-Brennan
- University of Liverpool, Liverpool, United Kingdom
- R.-D. Herzberg
- University of Liverpool, Liverpool, United Kingdom
- F. P. Heßberger
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- F. P. Heßberger
- Helmholtz-Institut Mainz, Mainz, Germany
- D. Hinde
- Australian National University, Canberra, ACT, Australia
- A. Hübner
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- D. Judson
- University of Liverpool, Liverpool, United Kingdom
- B. Kindler
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- Y. Komori
- RIKEN, Wako, Japan
- J. Konki
- 0University of Jyväskylä, Jyväskylä, Finland
- J.V. Kratz
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- N. Kurz
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Laatiaoui
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Laatiaoui
- Helmholtz-Institut Mainz, Mainz, Germany
- M. Laatiaoui
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- S. Lahiri
- 1Saha Institute of Nuclear Physics, Kolkata, India
- B. Lommel
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- M. Maiti
- 2Indian Institute of Technology Roorkee, Roorkee, India
- A. K. Mistry
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- A. K. Mistry
- Helmholtz-Institut Mainz, Mainz, Germany
- Ch. Mokry
- Helmholtz-Institut Mainz, Mainz, Germany
- Ch. Mokry
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- K. J. Moody
- Lawrence Livermore National Laboratory, Livermore, CA, United States
- Y. Nagame
- Japan Atomic Energy Agency, Tokai, Japan
- J. P. Omtvedt
- 3University of Oslo, Oslo, Norway
- P. Papadakis
- University of Liverpool, Liverpool, United Kingdom
- V. Pershina
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- D. Rudolph
- Lund University, Lund, Sweden
- L.G. Samiento
- Lund University, Lund, Sweden
- T.K. Sato
- Japan Atomic Energy Agency, Tokai, Japan
- M. Schädel
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- P. Scharrer
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- P. Scharrer
- Helmholtz-Institut Mainz, Mainz, Germany
- P. Scharrer
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- B. Schausten
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- D. A. Shaughnessy
- Lawrence Livermore National Laboratory, Livermore, CA, United States
- J. Steiner
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- P. Thörle-Pospiech
- Helmholtz-Institut Mainz, Mainz, Germany
- P. Thörle-Pospiech
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- A. Toyoshima
- Japan Atomic Energy Agency, Tokai, Japan
- N. Trautmann
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- K. Tsukada
- Japan Atomic Energy Agency, Tokai, Japan
- J. Uusitalo
- 0University of Jyväskylä, Jyväskylä, Finland
- K.-O. Voss
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- A. Ward
- University of Liverpool, Liverpool, United Kingdom
- M. Wegrzecki
- 4Łukasiewicz Research Network—Institute of Electron Technology, Warsaw, Poland
- N. Wiehl
- Helmholtz-Institut Mainz, Mainz, Germany
- N. Wiehl
- Johannes Gutenberg-Universität Mainz, Mainz, Germany
- E. Williams
- Australian National University, Canberra, ACT, Australia
- V. Yakusheva
- GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt, Germany
- V. Yakusheva
- Helmholtz-Institut Mainz, Mainz, Germany
- DOI
- https://doi.org/10.3389/fchem.2022.976635
- Journal volume & issue
-
Vol. 10
Abstract
Flerovium (Fl, element 114) is the heaviest element chemically studied so far. To date, its interaction with gold was investigated in two gas-solid chromatography experiments, which reported two different types of interaction, however, each based on the level of a few registered atoms only. Whereas noble-gas-like properties were suggested from the first experiment, the second one pointed at a volatile-metal-like character. Here, we present further experimental data on adsorption studies of Fl on silicon oxide and gold surfaces, accounting for the inhomogeneous nature of the surface, as it was used in the experiment and analyzed as part of the reported studies. We confirm that Fl is highly volatile and the least reactive member of group 14. Our experimental observations suggest that Fl exhibits lower reactivity towards Au than the volatile metal Hg, but higher reactivity than the noble gas Rn.
Keywords