Nature Communications (May 2023)

Correlated insulator collapse due to quantum avalanche via in-gap ladder states

  • Jong E. Han,
  • Camille Aron,
  • Xi Chen,
  • Ishiaka Mansaray,
  • Jae-Ho Han,
  • Ki-Seok Kim,
  • Michael Randle,
  • Jonathan P. Bird

DOI
https://doi.org/10.1038/s41467-023-38557-8
Journal volume & issue
Vol. 14, no. 1
pp. 1 – 8

Abstract

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Abstract The significant discrepancy observed between the predicted and experimental switching fields in correlated insulators under a DC electric field far-from-equilibrium necessitates a reevaluation of current microscopic understanding. Here we show that an electron avalanche can occur in the bulk limit of such insulators at arbitrarily small electric field by introducing a generic model of electrons coupled to an inelastic medium of phonons. The quantum avalanche arises by the generation of a ladder of in-gap states, created by a multi-phonon emission process. Hot-phonons in the avalanche trigger a premature and partial collapse of the correlated gap. The phonon spectrum dictates the existence of two-stage versus single-stage switching events which we associate with charge-density-wave and Mott resistive phase transitions, respectively. The behavior of electron and phonon temperatures, as well as the temperature dependence of the threshold fields, demonstrates how a crossover between the thermal and quantum switching scenarios emerges within a unified framework of the quantum avalanche.