Bidirectional to unidirectional emission of fluorescence controlled by optical traveling wave antennas

Abstract

Tailoring the fluorescence emission of quantum emitters to a desired direction is a crucial issue to achieve high efficient photodetection and realize unique optoelectronic devices. In this study, the directional emission of quantum dots controlled by optical traveling wave antennas based on 1D silver nanowires (NWs) was investigated. Both leaky waves and surface waves on a single NW are utilized for fluorescence emission control, and we show that the coupled fluorescence transforms from bidirectional to unidirectional emission when the surrounding medium changes from air to water. Moreover, in the unidirectional case, we obtain an ultra-narrow half-power bandwidth about 20°. Finite-difference time-domain simulations and Green’s function method in a stratified medium are used to calculate the far-field emission patterns of the hybrid structures, which agree well with the experiments. Further analyses based on typical modes and the dipole-chain model also reveal the mechanism behind the bidirectional and unidirectional fluorescence emission. These results show that the structures have great potential in integrated on-chip, sensing and photon-collection devices.

Keywords

• fluorescence emission
• nanoantennas
• bidirectional emission
• unidirectional fluorescence