Impact of aerosol–meteorology interactions on fine particle pollution during China’s severe haze episode in January 2013

Abstract

In January 2013, a severe regional haze occurred over the North China Plain. An online-coupled meteorology-chemistry model was employed to simulate the impacts of aerosol–meteorology interactions on fine particles (PM _2.5 ) pollution during this haze episode. The response of PM _2.5 to meteorology change constituted a feedback loop whereby planetary boundary layer (PBL) dynamics amplified the initial perturbation of PM _2.5 . High PM _2.5 concentrations caused a decrease of surface solar radiation. The maximal decrease in daily average solar radiation reached 53% in Beijing, thereby leading to a more stable PBL. The peak PBL height in Beijing decreased from 690 m to 590 m when the aerosol extinction was considered. Enhanced PBL stability suppressed the dispersion of air pollutants, and resulted in higher PM _2.5 concentrations. The maximal increase of PM _2.5 concentrations reached 140 μ g m ^−3 in Beijing. During most PM _2.5 episodes, primary and secondary particles increased simultaneously. These results imply that the aerosol–radiation interactions played an important role in the haze episode in January 2013.

Keywords

• meteorology
• fine particles
• aerosol–radiation interactions
• haze
• solar radiation