Nature Communications (Feb 2019)

High temperature singlet-based magnetism from Hund’s rule correlations

  • Lin Miao,
  • Rourav Basak,
  • Sheng Ran,
  • Yishuai Xu,
  • Erica Kotta,
  • Haowei He,
  • Jonathan D. Denlinger,
  • Yi-De Chuang,
  • Y. Zhao,
  • Z. Xu,
  • J. W. Lynn,
  • J. R. Jeffries,
  • S. R. Saha,
  • Ioannis Giannakis,
  • Pegor Aynajian,
  • Chang-Jong Kang,
  • Yilin Wang,
  • Gabriel Kotliar,
  • Nicholas P. Butch,
  • L. Andrew Wray

DOI
https://doi.org/10.1038/s41467-019-08497-3
Journal volume & issue
Vol. 10, no. 1
pp. 1 – 8

Abstract

Read online

Electrons in uranium-based materials are often on the border between localised and itinerant behaviour, which can lead to unusual magnetic behaviour. Here the authors combine experiment and theory to show that USb2 may be an unusually high temperature example of a singlet-ground-state magnet.