Environment International (Jul 2020)
Short- and medium-chain chlorinated paraffins in multi-environmental matrices in the Tibetan Plateau environment of China: A regional scale study
Abstract
Research on the environmental fate and behavior of short- and medium-chain chlorinated paraffins (SCCPs and MCCPs, respectively), especially in high-altitude remote mountain areas, has rarely been conducted. In this study, the distribution and profiles of SCCPs and MCCPs in soils, barks, needles, lichens, and mosses in the Tibetan Plateau area were investigated during the period from 2010 to 2016. The total CP concentrations in soils, barks, needles, lichens, and mosses increased with increasing altitude from 1983 to 5147 m a.s.l. (above sea level), covering a range of 1843.5 km × 370.6 km. Generally, the mean SCCP levels were higher than mean MCCP levels in different environmental matrices. Moreover, as-obtained linear relationships between CP concentrations in different environmental matrices and altitudes (p < 0.05) indicated that the mountain cold-trapping could affect the presence and congener patterns of both SCCPs and MCCPs in the Tibetan Plateau environment. C10−11 and C14 congener groups were found to be the dominant groups in SCCPs and MCCPs in the environmental samples, respectively. Finally, the back-trajectory model was employed to reveal the differences of the potential sources in different regions of the Tibetan Plateau.