APL Materials (Oct 2021)
Roadmap on organic–inorganic hybrid perovskite semiconductors and devices
- Lukas Schmidt-Mende,
- Vladimir Dyakonov,
- Selina Olthof,
- Feray Ünlü,
- Khan Moritz Trong Lê,
- Sanjay Mathur,
- Andrei D. Karabanov,
- Doru C. Lupascu,
- Laura M. Herz,
- Alexander Hinderhofer,
- Frank Schreiber,
- Alexey Chernikov,
- David A. Egger,
- Oleksandra Shargaieva,
- Caterina Cocchi,
- Eva Unger,
- Michael Saliba,
- Mahdi Malekshahi Byranvand,
- Martin Kroll,
- Frederik Nehm,
- Karl Leo,
- Alex Redinger,
- Julian Höcker,
- Thomas Kirchartz,
- Jonathan Warby,
- Emilio Gutierrez-Partida,
- Dieter Neher,
- Martin Stolterfoht,
- Uli Würfel,
- Moritz Unmüssig,
- Jan Herterich,
- Clemens Baretzky,
- John Mohanraj,
- Mukundan Thelakkat,
- Clément Maheu,
- Wolfram Jaegermann,
- Thomas Mayer,
- Janek Rieger,
- Thomas Fauster,
- Daniel Niesner,
- Fengjiu Yang,
- Steve Albrecht,
- Thomas Riedl,
- Azhar Fakharuddin,
- Maria Vasilopoulou,
- Yana Vaynzof,
- Davide Moia,
- Joachim Maier,
- Marius Franckevičius,
- Vidmantas Gulbinas,
- Ross A. Kerner,
- Lianfeng Zhao,
- Barry P. Rand,
- Nadja Glück,
- Thomas Bein,
- Fabio Matteocci,
- Luigi Angelo Castriotta,
- Aldo Di Carlo,
- Matthias Scheffler,
- Claudia Draxl
Affiliations
- Lukas Schmidt-Mende
- Department of Physics, University of Konstanz, Universitaetsstr. 10, 78457 Konstanz, Germany
- Vladimir Dyakonov
- Experimental Physics VI, University of Würzburg, Am Hubland, 97074 Würzburg, Germany
- Selina Olthof
- Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
- Feray Ünlü
- Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
- Khan Moritz Trong Lê
- Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
- Sanjay Mathur
- Department of Chemistry, University of Cologne, Greinstraße 4-6, 50939 Cologne, Germany
- Andrei D. Karabanov
- Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen, 45141 Essen, Germany
- Doru C. Lupascu
- Institute for Materials Science and Center for Nanointegration Duisburg-Essen (CENIDE), University of Duisburg-Essen, 45141 Essen, Germany
- Laura M. Herz
- Clarendon Laboratory, Department of Physics, University of Oxford, Parks Road, Oxford OX1 3PU, United Kingdom
- Alexander Hinderhofer
- Institute of Applied Physics, University of Tübingen, Auf der Morgenstelle 10, 72076 Tübingen, Germany
- Frank Schreiber
- Institute of Applied Physics, University of Tübingen, Auf der Morgenstelle 10, 72076 Tübingen, Germany
- Alexey Chernikov
- Department of Physics, University of Regensburg, 93053 Regensburg, Germany
- David A. Egger
- Department of Physics, Technical University of Munich, 85748 Garching, Germany
- Oleksandra Shargaieva
- Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
- Caterina Cocchi
- Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
- Eva Unger
- Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group ‘Hybrid Materials Formation and Scaling,’ Kekulestr. 5, 12489 Berlin, Germany
- Michael Saliba
- Carl von Ossietzky Universität Oldenburg, Institute of Physics, Carl-von-Ossietzky-Straße 9, 26129 Oldenburg, Germany
- Mahdi Malekshahi Byranvand
- Institute for Photovoltaics (ipv), University of Stuttgart, Pfaffenwaldring 47, 70569 Stuttgart, Germany and Helmholtz Young Investigator Group, lEK5-Photovoltaik, Forschungszentrum Jülich, 52425 Jülich, Germany
- Martin Kroll
- Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden, 01062 Dresden, Germany
- Frederik Nehm
- Department of Physics and Materials Science, University of Luxembourg, Luxembourg, Luxembourg
- Karl Leo
- Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP), Technische Universität Dresden, 01062 Dresden, Germany
- Alex Redinger
- Department of Physics and Materials Science, University of Luxembourg, Luxembourg, Luxembourg
- Julian Höcker
- Experimental Physics VI, University of Würzburg, Am Hubland, 97074 Würzburg, Germany
- Thomas Kirchartz
- IEK5-Photovoltaik, Forschungszentrum Jülich, 52425 Jülich, Germany and Faculty of Engineering and CENIDE, University of Duisburg-Essen, Carl-Benz-Str. 199, 47057 Duisburg, Germany
- Jonathan Warby
- Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
- Emilio Gutierrez-Partida
- Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
- Dieter Neher
- Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
- Martin Stolterfoht
- Institute of Physics and Astronomy, University of Potsdam, Karl-Liebknecht-Str. 24-25, D-14476 Potsdam-Golm, Germany
- Uli Würfel
- Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany
- Moritz Unmüssig
- Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany
- Jan Herterich
- Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany
- Clemens Baretzky
- Freiburg Materials Research Center (FMF), University of Freiburg, Stefan-Meier-Str. 21, 79104 Freiburg, Germany
- John Mohanraj
- Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth, 95440 Bayreuth, Germany
- Mukundan Thelakkat
- Applied Functional Polymers, Macromolecular Chemistry I, University of Bayreuth, 95440 Bayreuth, Germany
- Clément Maheu
- Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
- Wolfram Jaegermann
- Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
- Thomas Mayer
- Surface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Strasse 3, 64287 Darmstadt, Germany
- Janek Rieger
- Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Staudtstr. 7, 91058 Erlangen, Germany
- Thomas Fauster
- Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Staudtstr. 7, 91058 Erlangen, Germany
- Daniel Niesner
- Lehrstuhl für Festkörperphysik, Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Staudtstr. 7, 91058 Erlangen, Germany
- Fengjiu Yang
- Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells, 12489 Berlin, Germany
- Steve Albrecht
- Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Young Investigator Group Perovskite Tandem Solar Cells, 12489 Berlin, Germany
- Thomas Riedl
- Institute of Electronic Devices, University of Wuppertal, 42119 Wuppertal, Germany
- Azhar Fakharuddin
- Department of Physics, University of Konstanz, Universitaetsstr. 10, 78457 Konstanz, Germany
- Maria Vasilopoulou
- Institute of Nanoscience and Nanotechnology, National Center for Scientific Research Demokritos, 15341 Agia Paraskevi, Attica, Greece
- Yana Vaynzof
- Integrated Center for Applied Physics and Photonic Materials (IAPP) and Center for Advancing Electronics Dresden (cfaed), Technische Universität Dresden, Nöthnitzer Straße 61, 01187 Dresden, Germany
- Davide Moia
- Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569 Stuttgart, Germany
- Joachim Maier
- Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569 Stuttgart, Germany
- Marius Franckevičius
- Department of Molecular Compound Physics, Center for Physical Sciences and Technology (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, Lithuania
- Vidmantas Gulbinas
- Department of Molecular Compound Physics, Center for Physical Sciences and Technology (FTMC), Saulėtekio Avenue 3, Vilnius LT-10257, Lithuania
- Ross A. Kerner
- Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
- Lianfeng Zhao
- Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
- Barry P. Rand
- Department of Electrical Engineering, Princeton University, Princeton, New Jersey 08544, USA
- Nadja Glück
- Department of Chemistry, Ludwig-Maximilians-University Munich, Butenandtstr. 5-13, 81377 Munich, Germany
- Thomas Bein
- Department of Chemistry, Ludwig-Maximilians-University Munich, Butenandtstr. 5-13, 81377 Munich, Germany
- Fabio Matteocci
- CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy
- Luigi Angelo Castriotta
- CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy
- Aldo Di Carlo
- CHOSE—Centre for Hybrid and Organic Solar Energy, Department of Electronic Engineering, University of Rome Tor Vergata, Roma 00133, Italy
- Matthias Scheffler
- Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin, Zum Großen Windkanal 2, 12489 Berlin, Germany
- Claudia Draxl
- Physics Department and IRIS Adlershof, Humboldt-Universität zu Berlin, Zum Großen Windkanal 2, 12489 Berlin, Germany
- DOI
- https://doi.org/10.1063/5.0047616
- Journal volume & issue
-
Vol. 9,
no. 10
pp. 109202 – 109202-82
Abstract
Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.
