Ultrasonics Sonochemistry (May 2022)
Periodicity in ultrasonic atomization involving beads-fountain oscillations and mist generation: Effects of driving frequency
Abstract
Ultrasonic atomization induced by high driving frequency, generally on the order of 1 MHz or higher, could involve a liquid fountain in the form of a corrugated jet, or a chain of “beads” of submillimeter diameter in contact. This study concerns dynamics/instability of such beads fountain, observed under lower input power density (≤ 6 W/cm2) of the “flat” ultrasound transducer with a “regulating” nozzle equipped, exhibiting time-varying characteristics with certain periodicity. High-speed, high-resolution images are processed for quantitative elucidation: frequency analysis (fast Fourier transform) and time–frequency analysis (discrete wavelet transform) are employed, respectively, to evaluate dominant frequencies of beads-surface oscillations and to reveal factor(s) triggering mist emergence. The resulting time variation in the measured (or apparent) fountain structure, associated with the recurring-beads size scalable to the ultrasound wavelength, subsumes periodic nature predictable from simple physical modeling as well as principle. It is further found that such dynamics in (time-series data for) the fountain structure at given height(s) along a series of beads would signal “bursting” of liquid droplets emanating out of a highly deformed bead often followed by a cloud of tiny droplets, or mist. In particular, the bursting appears to be not a completely random phenomenon but should concur with the fountain periodicity with a limited extent of probability.