Nature Communications (Dec 2020)
Depth-dependent valence stratification driven by oxygen redox in lithium-rich layered oxide
- Jin Zhang,
- Qinchao Wang,
- Shaofeng Li,
- Zhisen Jiang,
- Sha Tan,
- Xuelong Wang,
- Kai Zhang,
- Qingxi Yuan,
- Sang-Jun Lee,
- Charles J. Titus,
- Kent D. Irwin,
- Dennis Nordlund,
- Jun-Sik Lee,
- Piero Pianetta,
- Xiqian Yu,
- Xianghui Xiao,
- Xiao-Qing Yang,
- Enyuan Hu,
- Yijin Liu
Affiliations
- Jin Zhang
- Beijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Science
- Qinchao Wang
- Chemistry Division, Brookhaven National Laboratory
- Shaofeng Li
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Zhisen Jiang
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Sha Tan
- Chemistry Division, Brookhaven National Laboratory
- Xuelong Wang
- Chemistry Division, Brookhaven National Laboratory
- Kai Zhang
- Beijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Science
- Qingxi Yuan
- Beijing Synchrotron Radiation Facility, Institute of High Energy Physics, Chinese Academy of Science
- Sang-Jun Lee
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Charles J. Titus
- Department of Physics, Stanford University
- Kent D. Irwin
- Department of Physics, Stanford University
- Dennis Nordlund
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Jun-Sik Lee
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Piero Pianetta
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- Xiqian Yu
- Beijing Advanced Innovation Center for Materials Genome Engineering, Key Laboratory for Renewable Energy, Beijing Key Laboratory for New Energy Materials and Devices, Institute of Physics, Chinese Academy of Sciences
- Xianghui Xiao
- National Synchrotron Light Source II, Brookhaven National Laboratory
- Xiao-Qing Yang
- Chemistry Division, Brookhaven National Laboratory
- Enyuan Hu
- Chemistry Division, Brookhaven National Laboratory
- Yijin Liu
- Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory
- DOI
- https://doi.org/10.1038/s41467-020-20198-w
- Journal volume & issue
-
Vol. 11,
no. 1
pp. 1 – 8
Abstract
Lithium-rich layered material deserves in-depth understanding because it has large capacity enabled by both cation and anion activities. Here, authors apply 3D spectro-tomography with nano resolution to reveal the multi-layer morphology and depth-dependent transition metal valence distribution associated with oxygen redox.