A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes

W. H. Li; C. J. R. Duncan; M. B. Andorf; A. C. Bartnik; E. Bianco; L. Cultrera; A. Galdi; M. Gordon; M. Kaemingk; C. A. Pennington; L. F. Kourkoutis; I. V. Bazarov; J. M. Maxson

doi:10.1063/4.0000138

Structural Dynamics (Mar 2022)

A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes

W. H. Li,
C. J. R. Duncan,
M. B. Andorf,
A. C. Bartnik,
E. Bianco,
L. Cultrera,
A. Galdi,
M. Gordon,
M. Kaemingk,
C. A. Pennington,
L. F. Kourkoutis,
I. V. Bazarov,
J. M. Maxson

Affiliations

W. H. Li: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
C. J. R. Duncan: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
M. B. Andorf: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
A. C. Bartnik: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
E. Bianco: Kavli Institute at Cornell for Nanoscale Science, Ithaca, New York 14853, USA
L. Cultrera: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
A. Galdi: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
M. Gordon: University of Chicago, Chicago, Illinois 60637, USA
M. Kaemingk: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
C. A. Pennington: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
L. F. Kourkoutis: Kavli Institute at Cornell for Nanoscale Science, Ithaca, New York 14853, USA
I. V. Bazarov: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA
J. M. Maxson: Cornell Laboratory for Accelerator-Based Sciences and Education, Cornell University, Ithaca, New York 14853, USA

DOI: https://doi.org/10.1063/4.0000138
Journal volume & issue: Vol. 9, no. 2
pp. 024302 – 024302-11

Abstract

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We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micrometer probe size, long coherence length, and 200 fs rms time resolution. We measure the 5d (peak) beam brightness at the sample location in micro-diffraction mode to be 7 × 10 13 A / m 2 rad 2. To generate high brightness electron bunches, the system employs high efficiency, low emittance semiconductor photocathodes driven with a wavelength near the photoemission threshold at a repetition rate up to 250 kHz. We characterize spatial, temporal, and reciprocal space resolution of the apparatus. We perform proof-of-principle measurements of ultrafast heating in single crystal Au samples and compare experimental results with simulations that account for the effects of multiple scattering.

Published in Structural Dynamics

ISSN: 2329-7778 (Online)
Publisher: AIP Publishing LLC and ACA
Country of publisher: United States
LCC subjects: Science: Chemistry: Crystallography
Website: http://sd.aip.org

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