Atmospheric Chemistry and Physics (Jun 2023)
Aerosol–cloud–radiation interaction during Saharan dust episodes: the dusty cirrus puzzle
Abstract
Dusty cirrus clouds are extended optically thick cirrocumulus decks that occur during strong mineral dust events. So far they have mostly been documented over Europe associated with dust-infused baroclinic storms. Since today's global numerical weather prediction models neither predict mineral dust distributions nor consider the interaction of dust with cloud microphysics, they cannot simulate this phenomenon. We postulate that the dusty cirrus forms through a mixing instability of moist clean air with drier dusty air. A corresponding sub-grid parameterization is suggested and tested in the ICOsahedral Nonhydrostatic model with Aerosol and Reactive Trace gases (ICON-ART). Only with the help of this parameterization is ICON-ART able to simulate the formation of the dusty cirrus, which leads to substantial improvements in cloud cover and radiative fluxes compared to simulations without this parameterization. A statistical evaluation over six Saharan dust events with and without observed dusty cirrus shows robust improvements in cloud and radiation scores. The ability to simulate dusty cirrus formation removes the linear dependency on mineral dust aerosol optical depth from the bias of the radiative fluxes. For the six Saharan dust episodes investigated in this study, the formation of dusty cirrus clouds is the dominant aerosol–cloud–radiation effect of mineral dust over Europe.