Regulating coordination number in atomically dispersed Pt species on defect-rich graphene for n-butane dehydrogenation reaction

Xiaowen Chen; Mi Peng; Xiangbin Cai; Yunlei Chen; Zhimin Jia; Yuchen Deng; Bingbao Mei; Zheng Jiang; Dequan Xiao; Xiaodong Wen; Ning Wang; Hongyang Liu; Ding Ma

doi:10.1038/s41467-021-22948-w

Nature Communications (May 2021)

Regulating coordination number in atomically dispersed Pt species on defect-rich graphene for n-butane dehydrogenation reaction

Xiaowen Chen,
Mi Peng,
Xiangbin Cai,
Yunlei Chen,
Zhimin Jia,
Yuchen Deng,
Bingbao Mei,
Zheng Jiang,
Dequan Xiao,
Xiaodong Wen,
Ning Wang,
Hongyang Liu,
Ding Ma

Affiliations

Xiaowen Chen: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Mi Peng: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
Xiangbin Cai: Department of Physics and Center for Quantum Materials, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon
Yunlei Chen: State Key Laboratory of Coal Conversion, Institute Coal Chemistry, Chinese Academy of Sciences
Zhimin Jia: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Yuchen Deng: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University
Bingbao Mei: Shanghai Institute of Applied Physics, Chinese Academy of Sciences
Zheng Jiang: Shanghai Institute of Applied Physics, Chinese Academy of Sciences
Dequan Xiao: Center for Integrative Materials Discovery, Department of Chemistry and Chemical Engineering, University of New Haven
Xiaodong Wen: State Key Laboratory of Coal Conversion, Institute Coal Chemistry, Chinese Academy of Sciences
Ning Wang: Department of Physics and Center for Quantum Materials, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon
Hongyang Liu: Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences
Ding Ma: Beijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking University

DOI: https://doi.org/10.1038/s41467-021-22948-w
Journal volume & issue: Vol. 12, no. 1
pp. 1 – 9

Abstract

Read online

Direct dehydrogenation has been a thematic research area resulting from the energy shortage and petroleum gas upgrading scenario. Here, the authors fabricate fully exposed Pt3 clusters and correlate dehydrogenation activity with average coordination number of Pt-Pt bond.

Published in Nature Communications

ISSN: 2041-1723 (Online)
Publisher: Nature Portfolio
Country of publisher: United Kingdom
LCC subjects: Science
Website: https://www.nature.com/ncomms/

About the journal