The Aerosol-Radiation Interaction Effects of Different Particulate Matter Components during Heavy Pollution Periods in China

Abstract

: The Beijing-Tianjin-Hebei (BTH) region experienced heavy air pollution in December 2015, which provided a good opportunity to explore the aerosol-radiation interaction (ARI) effects of different particulate matter (PM) components (sulfate, nitrate, and black carbon (BC)). In this study, five tests were conducted by the Weather Research and Forecasting—Chemistry (WRF-Chem) model. The tests included scenario 1 simulation with ARI turned on, scenario 2 simulation with ARI turned off, scenario3 simulation without NOx/NO3- emissions and with ARI turned on, scenario 4 simulation without SO2/SO42− emissions and with ARI turned on, and scenario 5 simulation without BC emissions and with ARI turned on. The ARI decreased the downward shortwave radiation (SWDOWN) and the temperature at 2 m (T2), reduced the planetary boundary layer (PBL) height (PBLH), and increased the relative humidity (RH) at 2 m in the region. These factors also contribute to pollution accumulation. The results revealed that BC aerosols have a stronger effect on the reduction in SWDOWN than sulfate (SO42−) and nitrate (NO3−). BC aerosols produce both cooling and heating effects, while SO42− aerosols produce only cooling effects. The PBL decreased and RH2 increased due to the aerosol feedback effect of sulfate, nitrate, and BC. The ARI effect on meteorological factors during the nonheavy pollution period was much smaller than that during the pollution period.

Keywords

• aerosol-radiation interaction
• black carbon
• sulfate aerosols
• nitrate aerosols
• meteorological factors