Nano-Micro Letters (Jun 2024)
Polymer Fiber Rigid Network with High Glass Transition Temperature Reinforces Stability of Organic Photovoltaics
- Qiao Zhou,
- Cenqi Yan,
- Hongxiang Li,
- Zhendong Zhu,
- Yujie Gao,
- Jie Xiong,
- Hua Tang,
- Can Zhu,
- Hailin Yu,
- Sandra P. Gonzalez Lopez,
- Jiayu Wang,
- Meng Qin,
- Jianshu Li,
- Longbo Luo,
- Xiangyang Liu,
- Jiaqiang Qin,
- Shirong Lu,
- Lei Meng,
- Frédéric Laquai,
- Yongfang Li,
- Pei Cheng
Affiliations
- Qiao Zhou
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Cenqi Yan
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Hongxiang Li
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Zhendong Zhu
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Yujie Gao
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Jie Xiong
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Hua Tang
- KAUST Solar Center, Physical Science and Engineering Division, King Abdullah University of Science and Technology (KAUST)
- Can Zhu
- Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences
- Hailin Yu
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Sandra P. Gonzalez Lopez
- KAUST Solar Center, Physical Science and Engineering Division, King Abdullah University of Science and Technology (KAUST)
- Jiayu Wang
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Meng Qin
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Jianshu Li
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Longbo Luo
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Xiangyang Liu
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Jiaqiang Qin
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- Shirong Lu
- Department of Material Science and Technology, Taizhou University
- Lei Meng
- Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences
- Frédéric Laquai
- KAUST Solar Center, Physical Science and Engineering Division, King Abdullah University of Science and Technology (KAUST)
- Yongfang Li
- Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences
- Pei Cheng
- College of Polymer Science and Engineering, State Key Laboratory of Polymer Materials Engineering, Sichuan University
- DOI
- https://doi.org/10.1007/s40820-024-01442-0
- Journal volume & issue
-
Vol. 16,
no. 1
pp. 1 – 14
Abstract
Highlights A unique approach is proposed: constructing a polymer fiber rigid network with high glass transition temperature. Frozen bulk heterojunction morphology impeded deterioration of exciton quenching, charge transport, and charge extraction properties during thermal aging. The strategy is universal and can be further optimized for enhanced thermal stability and improved mechanical resilience.
Keywords
- Inverted organic photovoltaics
- Thermal stability
- Aramid nanofibers
- Morphology control
- Charge carrier dynamics
